You can almost certainly fit the /R, S3 or TTS brakes onto your TT. I say almost because I know nothing about the stock wheels on the TT. To answer that question I'd probably head over the Vortex and see what wheel setups the /R folks are using.
To your question, OE upgrade or BBK, it depends on what your goals are. If you're just looking to fill out the wheel and make it look sexy, the TTS setup will do you very nicely. In fact, if that's where you want to go I have a set of TTS front calipers I'll sell you cheap, you'll just have rebuild them. :-P . If you desire performance then I would definitely NOT recommend the TTS setup as it's unique to the TTS alone and there's not any aftermarket suppliers at the moment so you're stuck with OE rotors and pads which are, to put it nicely, a tad expensive for the performance they provide. Put another way, for true performance braking you should definitely go with a BBK.
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